专题论文

膜分离技术在放射性废水处理中的应用

  • 张雅琴 ,
  • 张林 ,
  • 侯立安
展开
  • 1. 浙江大学化学工程与生物工程学院, 杭州310027;
    2. 第二炮兵工程大学3系, 西安710025
张雅琴,博士研究生,研究方向为膜法水处理,电子信箱:yaqin0626@163.com

收稿日期: 2015-05-03

  修回日期: 2015-06-02

  网络出版日期: 2015-08-14

基金资助

国家自然科学基金项目(51238006,L1422037);中国工程科技中长期发展战略研究项目(2014-zcp-10)

Application of membrane technology in liquid radioactive waste processing

  • ZHANG Yaqin ,
  • ZHANG Lin ,
  • HOU Li'an
Expand
  • 1. College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China;
    2. Xi'an High-Tech Institute, Xi'an 710025, China

Received date: 2015-05-03

  Revised date: 2015-06-02

  Online published: 2015-08-14

摘要

涉核技术的快速发展和应用领域的扩展,对放射性废水的处理提出了更高的要求,膜分离技术在放射性废水处理方面表现出良好的应用前景。本文简述了微滤、超滤、纳滤、反渗透、电渗析、膜蒸馏及液膜等膜过程处理放射性废水的机制,综述了国内外膜法处理放射性废水的应用及研究现状,探讨了膜分离技术应用中存在的问题及发展方向。

本文引用格式

张雅琴 , 张林 , 侯立安 . 膜分离技术在放射性废水处理中的应用[J]. 科技导报, 2015 , 33(14) : 24 -27 . DOI: 10.3981/j.issn.1000-7857.2015.14.003

Abstract

The liquid radioactive waste treatment is a challenging task in the rapid development and extensive applications of nuclear technology. The membrane technologies have a potential application in the liquid radioactive waste treatment. In this paper, the mechanisms of different membrane processes to treat the liquid radioactive waste, including the microfiltration, the ultrafiltration, the nanofiltration, the reverseosmosis, the electrodialysis, the membrane distillation, and the liquid membrane process, are reviewed. The application and the research progress of the membrane treatment of the liquid radioactive waste water at home and abroad are discussed in detail, and the new directions and the existing problems of the membrane technology in the field are pointed out.

参考文献

[1] Rahman R O A, Ibrahium H A, Hung Y T. Liquid radioactive wastes treatment: A review[J]. Water, 2011, 3(2): 551-65.
[2] Rana D, Matsuura T, Kassim M A, et al. Radioactive decontamination of water by membrane processes: A review[J]. Desalination, 2013, 321: 77-92.
[3] 刘萍, 曾光明, 黄瑾辉, 等. 膜技术在饮用水深度处理上的应用[J]. 环 境科学与技术, 2004, 27(6): 100-103. Liu Ping, Zeng Guangming, Huang Jinhui, et al. Application of membrane technology in advanced treatment of drinking water[J]. Environmental Science & Technology, 2004, 27(6): 100-103.
[4] Kryvoruchko A P, Yu L, Atamanenko I D, et al. Ultrafiltration removal of U(VI) from contaminated water[J]. Desalination, 2004, 162(1-3): 229- 236.
[5] 孔劲松, 王晓伟, 姚青旭. 含活化产物放射性废水的胶束强化超滤处 理研究[J]. 核动力工程, 2012, 33(4): 127-130. Kong Jinsong, Wang Xiaowei, Yao Qingxu. Study on treatment of radioactive wastewater containing activated products by micellarenhanced ultrafiltration process[J]. Nuclear Power Engineering, 2012, 33 (4): 127-130.
[6] 侯立安. 核沾染水处理技术及饮用水安全保障[J]. 给水排水, 2011, 37 (11): 1-3. Hou Li'an. Nuclear contamination of water treatment technology and drinking water security[J]. Water & Wastewater Engineering, 2011, 37 (11): 1-3.
[7] Astruc C, Baumgartner C, Bonneau S, et al. Filtration in nuclear power plants[C]. Euromembrane 99, Leuven, Belgium, September 19-22, 1999.
[8] 侯立安, 左莉. 纳滤膜分离技术处理放射性污染废水的试验研究[J]. 给水排水, 2004, 30(10): 47-49. Hou Li'an, Zuo Li. erimental research on nano-membrane filtration for radioactive contaminated wastewater treatment[J]. Water & Wastewater Engineering, 2004, 30(10): 47-49.
[9] 侯立安, 左莉, 刘晓敏, 等. 纳滤和离子交换组合工艺去除模拟核及生 物毒剂废水的试验研究[C]. 第二届中国膜科学与技术报告会, 北京, 09-13-15, 2005. Hou Li'an, Zuo Li, Liu Xiaomin, et al. Experimental study on combined process of removal of simulated nuclear and biological agents and ion exchange wastewater by nanofiltration[C]. Second China Membrane Science and Technology Report, Beijing, September 13-15, 2005.
[10] 张维润, 樊雄. 膜分离技术处理放射性废水[J]. 水处理技术, 2009, 35 (10): 1-5. Zhang Weirun, Fan Xiong. Treatment of radioactive wastewater by membrane separation technology[J]. Technology of Water Treatment, 2009, 35(10): 1-5.
[11] 杜志辉, 贾铭椿, 王晓伟. 复合反渗透膜对模拟放射性核素的截留性 能研究[J]. 武汉理工大学学报: 交通科学与工程版, 2012, 36(1): 180-183. Du Zhihui, Jia Mingchun, Wang Xiaowei. Study on Rejection Performance of Composite Reverse Osmosis Membrane to Simulated Radionuclide[J]. Journal of Wuhan University of Technology: Transportation Science & Engineering, 2012, 36(1): 180-183.
[12] Chmielewski A G, Harasimowicz M, Tyminski B, et al. Concentration of low- and medium-level radioactive wastes with three-stage reverse osmosis pilot plant[J]. Separation Science and Technology, 20013, 6(5/ 6): 1117-1127.
[13] Sengupta S K, Buckley L P, Rimpelainen S, et al. Liquid rad waste processing with spiral wound reverse osmosis[R]. Chalk River Atomic Energy of Canada Limited, AECL Report, No.11542, 1996 .
[14] Tan L, Tapsell G. Operation of a membrane pilot plant for ANSTO effluent[C/OL]. [2015-01-31]. http://www.wmsym.org/archives/2004/ pdfs/4194.pdf.
[15] Zakrzewska-Trznadel G, Harasimowicz M, Chmielewski A G. Membrane processes innuclear technology-application for liquid radioactive waste treatment[J]. Separation and Purification Technology, 2001, 22: 617-25.
[16] Lundstrom J E. Decontamination of a radioactive waste liquid by electrodialysis: US Patent 4645625[P]. 1987-02-24.
[17] Gasser M. S, Nowier H G. Separation of strontium and cadmiumions from nitrate medium by ion-exchange membrane in an electrodialysis system[J]. Journal of Chemical Technology and Biotechnology, 2004, 79 (1): 97-102.
[18] Neville M D, Jones C P, Turner A D. The EIX process for radioactive wastet reatment[J]. Progress in Nuclear Energy, 1998, 32(3/4): 397- 401.
[19] Zakrzewska-Trznadel G, Harasimowicz M, Chmielewski A G. Concentration of radioactive components in liquid low-level radioactive waste by membrane distillation[J]. Journal of Membrane Science, 1999, 163(2): 257-264.
[20] Teramoto M, Fu S S, Takatani K, et al. Treatment of simulated low level radioactive waste water by supported liquid membranes: Uphilltran sport of Ce (III) using CMPO ascarrier[J]. Separation and purification technology, 1999, 18(1): 57-69.
文章导航

/